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北祁连甘肃毛藏寺铜-钼矿床花岗质岩石锆石U-Pb年龄、地球化学特征及其地质意义

赵辛敏, 郭周平, 王育习, 高永伟, 张乐, 白赟, 杨生飞

赵辛敏, 郭周平, 王育习, 高永伟, 张乐, 白赟, 杨生飞. 2018: 北祁连甘肃毛藏寺铜-钼矿床花岗质岩石锆石U-Pb年龄、地球化学特征及其地质意义. 地质通报, 37(4): 669-681.
引用本文: 赵辛敏, 郭周平, 王育习, 高永伟, 张乐, 白赟, 杨生飞. 2018: 北祁连甘肃毛藏寺铜-钼矿床花岗质岩石锆石U-Pb年龄、地球化学特征及其地质意义. 地质通报, 37(4): 669-681.
ZHAO Xinmin, GUO Zhouping, WANG Yuxi, GAO Yongwei, ZHANG Le, BAI Yun, YANG Shengfei. 2018: Zircon U-Pb age, geochemical characteristics and geo-logical significance of granitoids in the Maozangsi deposit, Northern Qilian Mountain. Geological Bulletin of China, 37(4): 669-681.
Citation: ZHAO Xinmin, GUO Zhouping, WANG Yuxi, GAO Yongwei, ZHANG Le, BAI Yun, YANG Shengfei. 2018: Zircon U-Pb age, geochemical characteristics and geo-logical significance of granitoids in the Maozangsi deposit, Northern Qilian Mountain. Geological Bulletin of China, 37(4): 669-681.

北祁连甘肃毛藏寺铜-钼矿床花岗质岩石锆石U-Pb年龄、地球化学特征及其地质意义

基金项目: 

中国地质调查局项目《祁连成矿带肃南—大柴旦地区地质矿产调查》 DD20160012

详细信息
    作者简介:

    赵辛敏(1988-), 男, 硕士, 研究实习员, 从事矿床地球化学研究。E-mail:835177076@qq.com

  • 中图分类号: P597+.3;P618.41;P618.65

Zircon U-Pb age, geochemical characteristics and geo-logical significance of granitoids in the Maozangsi deposit, Northern Qilian Mountain

  • 摘要:

    甘肃毛藏寺铜钼矿是与花岗质岩石有关的斑岩型矿床,矿区内花岗质岩石类型主要为似斑状二长花岗岩和花岗闪长岩。对矿区岩体进行年龄、地球化学研究,以约束其形成时代,并探讨岩石成因及其与成矿的关系。LA-ICP-MS锆石UPb测年分别获得似斑状二长花岗岩与花岗闪长岩谐和年龄为455.8±3.1Ma和425.0±2.8Ma,属于晚奥陶世和晚志留世岩浆活动的产物。地球化学数据显示,似斑状二长花岗岩属于过铝质钙碱性岩浆系列,花岗闪长岩属于准铝质高钾钙碱性岩浆系列,二者均富集大离子亲石元素,亏损高场强元素,稀土元素配分曲线呈右倾型,轻、重稀土元素分馏明显。似斑状二长花岗岩具有弱正Eu异常(δEu=1.18~1.24),显示埃达克岩的地球化学特征,形成于北祁连洋俯冲消减阶段,由俯冲洋壳(含海洋沉积物)部分熔融形成,源区主要残留物为石榴子石。花岗闪长岩显示弱负Eu异常,形成于碰撞后伸展环境,是洋壳板片断离后软流圈上涌诱发的下地壳玄武质岩石部分熔融的产物。似斑状二长花岗岩符合成矿期埃达克岩特征,具有较好的成矿条件。结合前人资料,在北祁连东段寻找和勘查与埃达克岩有关的铜-钼-金矿可能是一个新的方向。

    Abstract:

    The Maozangsi Cu-Mo deposit in Gansu is a porphyry type deposit related to granitoids. Maozangsi granitoids are com-posed of porphyritoid monzogranite and granodiorite. In this paper, zircon U-Pb dating and geochemical study of the Maozangsi granitoids were conducted to constrain its geochronology and discuss petrogenesis and its relationship with mineralization. Zircon LA-ICP-MS dating yielded concordant ages of 455.8±3.1Ma and 425.0±2.8Ma respectively, indicating that the two plutons were formed in Late Ordovician and late Silurian respectively. Geochemical data show that porphyritoid monzogranite is a peraluminous granite and belongs to the calc-alkaline series, whereas granodiorite is a aluminous granite and belongs to the high-K calc-alkaline series. They are characterized by enrichment of LILEs and depletion of HFSEs, with REE patterns exhibiting the right-deviation type and strong fractionation with LREE enrichment. The porphyritoid monzogranite show weak positive Eu anomalies (δEu=1.18~1.24) and geochemical affinity to adakite, probably resulting from the slab melting (including marine sediments) of the subduction of North Qilian Ocean with the residual minerals of garnet in the source. The granodiorite shows weak negative Eu anomalies and was generated in a post-collisional extension setting and derived from partial melting of basaltic rocks in the lower crust induced by asthe-nosphere after the breakup of previously subducted North Qilian oceanic slab. The features of porphyritoid monzogranite are in ac-cordance with the characteristics of ore-forming period adakitic rocks and thus suggest good mineralization conditions. In combina-tion with data obtained from previous studies, the authors hold that it is possible to find Cu-Mo-Au deposits related to adakites in the eastern section of the Northern Qilian Mountain.

  • 致谢: 衷心感谢中国地质调查局西安地质调查中心杨合群研究员在成文过程中给予的帮助和指导。
  • 图  1   北祁连山地质简图[18]

    1—中新生界;2—晚古生代沉积岩系;3—寒武纪复理石建造;4—奥陶纪火山岩系;5—中寒武世-早奥陶世火山岩系;6—前寒武系;7—前加里东期花岗岩类;8—加里东期花岗岩类;9—加里东期后花岗岩类

    Figure  1.   Geological sketch map of Northern Qilian Mountain

    图版Ⅰ   a.似斑状二长花岗岩;b.花岗闪长岩;c.钾长石化、绢云母化铜钼矿石;d.浸染状铜钼矿石;e、f.黄铜矿-辉钼矿-石英脉

    图  2   毛藏寺矿区二长花岗岩(a)和花岗闪长岩(b)锆石阴极发光(CL)图像

    Figure  2.   Zircon CL images of the monzogranite (a) and granodiorite (b) from the Maozangsi deposit

    图  3   毛藏寺矿区二长花岗岩(a)和花岗闪长岩(b)锆石U-Pb谐和图

    Figure  3.   Zircon U-Pb concordia diagrams for the monzogranite (a) and granodiorite (b) from the Maozangsi deposit

    图  4   毛藏寺矿区花岗质岩石SiO2-K2O[20](a)及A/CNK-A/NK图解[21](b)

    Figure  4.   SiO2-K2O (a) and A/CNK-A/NK (b) diagrams of the granitoids from the Maozangsi deposit

    图  5   毛藏寺矿区花岗质岩石微量元素原始地幔标准化蛛网图(a)及稀土元素球粒陨石标准化配分曲线(b)(标准值据参考文献[22])

    Figure  5.   Primitive mantle-normalized trace element patterns (a) and chondrite-normalized REE patterns (b) of granitoids from the Maozangsi deposit

    图  6   毛藏寺矿区二长花岗岩和花岗闪长岩的Y-Sr/Y(a)和YbN-(La/Yb)N(b)图解

    Figure  6.   Y-Sr/Y(a) and YbN-(La/Yb)N(b) diagrams of the monzogranite and granodiorite from the Maozangsi deposit

    图  7   毛藏寺矿区埃达克岩地球化学特征图解(底图据参考文献[38])

    Figure  7.   Geochemical characteristics of adakites in the Maozangsi deposit

    图  8   毛藏寺矿区埃达克岩的Th/Sm-Th/Yb图解(N-MORB(正常洋中脊玄武岩)据参考文献[22];GLOSS(全球俯冲沉积物)据参考文献[40])

    Figure  8.   Th/Yb versus Th/Sm diagram for the adakite in the Maozangsi deposit

    图  9   毛藏寺矿区花岗质岩石(Y+Nb)-Rb图解(据参考文献[44])

    ORG—洋中脊花岗岩;VAG—火山弧花岗岩;WPG—板内花岗岩;Syn-COLG—同碰撞花岗岩;Post-COLG—后碰撞花岗岩

    Figure  9.   (Y+Nb)-Rb diagram for the granites in the Maozangsi deposit

    表  1   毛藏寺矿区花岗质岩石LA-ICP-MS锆石U-Th-Pb分析结果

    Table  1   LA-ICP-MS zircon U-Th-Pb isotopic data of Maozangsi granitoids

    测试点 Pb Th U Th/
    U
    207Pb/206Pb 207Pb/235U 206Pb/238U 207Pb/206Pb 207Pb/235U 206Pb/238U
    /lO-6 比值 比值 比值 年龄/
    Ma
    年龄/
    Ma
    年龄/
    Ma
    MZS1,二长花岗岩,16个测点(不包括3、8、19、20测点)
    MZS1-01 292 800 861 0.93 0.0522 0.0025 0.5515 0.0257 0.0766 0.0014 295.3 105.7 446.0 16.8 475.7 8.4
    MZS1-02 217 430 671 0.64 0.0664 0.0033 0.6687 0.0322 0.0730 0.0015 819.0 101.1 519.9 19.6 454.4 9.0
    MZS1-04 783 2934 2413 1.22 0.0555 0.0018 0.5606 0.0179 0.0732 0.0012 432.8 71.1 451.9 11.7 455.6 6.9
    MZS1-05 1032 1169 3171 0.37 0.0541 0.0014 0.5485 0.0140 0.0735 0.0010 376.1 56.8 444.0 9.2 457.2 6.3
    MZS1-06 602 1051 1765 0.60 0.0551 0.0018 0.5852 0.0189 0.0770 0.0012 416.8 71.4 467.8 12.1 478.2 7.2
    MZS1-07 883 2150 2569 0.84 0.0592 0.0016 0.6331 0.0167 0.0776 0.0011 572.7 57.1 498.0 10.4 477.9 6.8
    MZS1-09 466 1007 1434 0.70 0.0599 0.0017 0.6067 0.0174 0.0734 0.0011 601.2 61.7 481.5 11.0 456.7 6.6
    MZS1-10 766 2017 2351 0.86 0.0554 0.0011 0.5619 0.0116 0.0736 0.0010 427.1 44.4 452.8 7.6 457.8 5.8
    MZS1-11 1328 2711 4087 0.66 0.0559 0.0009 0.5662 0.0095 0.0735 0.0009 447.2 34.9 455.5 6.2 457.1 5.6
    MZS1-12 474 863 1479 0.58 0.0591 0.0014 0.5909 0.0137 0.0725 0.0010 570.7 49.5 471.4 8.7 451.3 6.0
    MZS1-13 1233 2057 3849 0.53 0.0563 0.0009 0.5630 0.0094 0.0725 0.0009 465.2 35.1 453.5 6.1 451.0 5.5
    MZS1-14 660 2418 2064 1.17 0.0578 0.0018 0.5759 0.0171 0.0723 0.0011 520.9 65.2 461.8 11.0 450.0 6.6
    MZS1-15 530 1055 1622 0.65 0.0559 0.0019 0.5700 0.0188 0.0740 0.0012 447.4 73.2 458.0 12.1 460.1 7.0
    MZS1-16 769 1269 2354 0.54 0.0682 0.0024 0.6949 0.0240 0.0739 0.0013 875.0 72.3 535.8 14.4 459.5 7.7
    MZS1-17 744 1732 2288 0.76 0.0527 0.0014 0.5347 0.0136 0.0736 0.0010 315.6 57.0 434.9 9.0 457.8 6.2
    MZS1-18 567 2138 1750 1.22 0.0551 0.0017 0.5571 0.0169 0.0734 0.0011 415.2 67.1 449.7 11.0 456.4 6.7
    MZS2,花岗闪长岩,18个测点(不包括11、15测点)
    MZS2-01 507 1584 1677 0.94 0.0569 0.0013 0.5373 0.0126 0.0685 0.0009 487.4 50.8 436.6 8.3 426.9 5.6
    MZS2-02 524 2087 1735 1.20 0.0549 0.0014 0.5180 0.0132 0.0684 0.0010 408.0 55.5 423.8 8.8 426.7 5.8
    MZS2-03 476 1550 1574 0.98 0.0532 0.0014 0.5030 0.0129 0.0685 0.0010 338.5 57.3 413.7 8.7 427.3 5.7
    MZS2-04 425 1681 1406 1.20 0.0564 0.0016 0.5324 0.0149 0.0685 0.0010 466.3 61.6 433.4 9.9 427.1 5.9
    MZS2-05 266 864 891 0.97 0.0547 0.0023 0.5113 0.0215 0.0678 0.0011 400.1 93.4 419.3 14.4 422.7 6.8
    MZS2-06 409 1192 1358 0.88 0.0576 0.0016 0.5416 0.0146 0.0682 0.0010 513.4 59.1 439.5 9.6 425.4 5.9
    MZS2-07 403 838 1340 0.63 0.0513 0.0019 0.4823 0.0175 0.0682 0.0011 253.6 83.1 399.6 12.0 425.3 6.6
    MZS2-08 372 1195 1249 0.96 0.0553 0.0019 0.5157 0.0170 0.0676 0.0010 424.6 72.8 422.3 11.4 421.8 6.2
    MZS2-09 382 1183 1287 0.92 0.0636 0.0017 0.5906 0.0154 0.0674 0.0010 727.6 54.8 471.3 9.8 420.3 5.8
    MZS2-10 632 2344 2112 1.11 0.0607 0.0012 0.5677 0.0116 0.0679 0.0009 627.7 42.7 456.6 7.5 423.3 5.4
    MZS2-12 274 906 923 0.98 0.0603 0.0018 0.5608 0.0166 0.0675 0.0010 614.1 63.4 452.0 10.8 420.8 6.0
    MZS2-13 402 1354 1346 1.01 0.0566 0.0015 0.5297 0.0138 0.0678 0.0009 476.5 57.0 431.6 9.2 423.1 5.7
    MZS2-14 492 1622 1643 0.99 0.0544 0.0013 0.5107 0.0125 0.0680 0.0009 389.2 54.0 418.9 8.4 424.3 5.6
    MZS2-16 194 582 643 0.90 0.0685 0.0028 0.6457 0.0260 0.0684 0.0012 883.8 83.5 505.8 16.0 426.3 7.3
    MZS2-17 499 1525 1649 0.92 0.0568 0.0013 0.5388 0.0122 0.0688 0.0009 483.2 49.1 437.6 8.0 428.9 5.6
    MZS2-18 414 1238 1379 0.90 0.0660 0.0018 0.6212 0.0164 0.0683 0.0010 806.3 55.0 490.6 10.3 425.7 6.0
    MZS2-19 434 1377 1446 0.95 0.0533 0.0014 0.5010 0.0132 0.0682 0.0009 341.2 58.9 412.4 8.9 425.2 5.6
    MZS2-20 450 2068 1491 1.39 0.0541 0.0014 0.5111 0.0129 0.0686 0.0009 373.6 55.6 419.2 8.7 427.5 5.7
    下载: 导出CSV

    表  2   毛藏寺矿区花岗质岩石的主量、微量和稀土元素分析结果

    Table  2   Major, trace and rare earth element data of the granitoids from the Maozangsi deposit

    样品号 MZ-7 MZ-8 MZ-9 MZ-10 MZ-11 MZ-12 MZ-18 MZ-19 MZ-20 MZ-21 MZ-22
    岩性 似斑状二长花岗岩 花岗闪长岩
    SiO2 70.67 71.04 70.76 70.94 71.07 70.26 63.02 63.36 63.16 63.12 62.99
    Al2O3 15.14 15.01 15.17 15.15 15.09 15.18 15.57 15.63 15.74 15.69 15.55
    Fe2O3 0.52 0.47 0.68 0.86 0.51 1.00 1.34 1.22 1.35 1.32 1.38
    FeO 1.18 1.15 0.87 0.82 1.25 0.91 3.28 3.22 3.17 3.22 3.25
    CaO 1.59 1.56 1.91 1.97 1.50 2.12 4.08 4.04 4.01 4.13 4.06
    MgO 0.94 0.86 0.74 0.75 0.81 0.73 3.31 3.18 3.26 3.23 3.47
    K2O 2.67 2.72 2.43 2.47 2.66 2.46 2.89 2.97 2.96 2.97 2.89
    Na2O 4.97 4.86 4.78 4.43 4.8 4.39 3.72 3.77 3.75 3.78 3.71
    TiO2 0.24 0.24 0.24 0.24 0.24 0.25 0.75 0.74 0.74 0.75 0.76
    P2O5 0.10 0.11 0.10 0.10 0.10 0.10 0.24 0.24 0.24 0.24 0.25
    MnO 0.06 0.06 0.05 0.05 0.06 0.06 0.08 0.08 0.08 0.08 0.08
    烧失量 1.86 1.87 2.20 2.18 1.83 2.48 1.60 1.47 1.45 1.39 1.51
    总计 99.94 99.95 99.93 99.96 99.92 99.94 99.88 99.92 99.91 99.92 99.90
    K2O+Na2O 7.64 7.58 7.21 6.90 7.46 6.85 6.61 6.74 6.71 6.75 6.60
    K2O/Na2O 0.54 0.56 0.51 0.56 0.55 0.56 0.78 0.79 0.79 0.79 0.78
    Mg# 0.51 0.50 0.47 0.46 0.46 0.42 0.57 0.57 0.57 0.57 0.58
    A/CNK 1.08 1.09 1.09 1.12 1.12 1.10 0.93 0.93 0.94 0.92 0.93
    DI 88.11 88.35 87.46 86.93 88.39 86.07 69.51 70.28 69.91 69.89 69.25
    Cu 65.7 90.5 159 38.7 104 16.6 67.9 46.1 60.5 43.9 56.8
    Pb 35.1 29.0 19.8 19.7 22.1 20.1 19.1 18.0 18.9 20.1 18.0
    Zn 82.7 63.4 50.4 49.5 57.8 50.1 85.4 71.8 78.7 72.2 81.1
    Cr 18.7 13.1 11.8 10.0 10.8 9.82 75.6 71.5 74.0 76.2 85.5
    Ni 14.2 6.26 5.62 5.41 5.82 6.65 47.0 43.2 46.6 46.8 56.6
    Co 3.54 3.36 3.04 3.43 3.12 4.13 15.5 14.8 15.4 15.9 16.3
    Li 15.9 16.1 10.1 10.2 10.7 11.0 22.3 20.8 21.2 20.2 22.5
    Rb 62.8 72.6 88.4 71.3 71.3 80.7 108 65.6 68.8 75.6 85.5
    Cs 3.67 4.56 3.36 3.98 4.21 4.17 4.81 4.19 4.43 4.39 4.57
    W 23.6 14.6 60.1 55.8 11.7 40.9 14.0 7.58 9.43 3.27 10.8
    Mo 0.27 0.30 0.51 0.52 0.55 0.61 1.31 1.12 1.11 0.94 1.22
    Bi 0.22 0.12 0.14 0.12 0.30 0.20 0.38 0.58 0.9 0.42 0.31
    Sr 520 582 396 457 526 556 691 615 613 674 704
    Ba 1540 1300 1170 1100 1180 996 1100 1010 998 1070 978
    V 24.2 24.0 24.1 23.2 25.1 24.9 109 104 107 108 111
    Sc 11.8 11.8 10.2 9.26 10.0 10.4 17.1 15.6 15.1 13.8 14.9
    Nb 4.49 4.22 4.30 5.06 3.98 4.75 12.1 10.9 10.9 11.6 11.6
    Ta 0.36 0.34 0.39 0.41 0.35 0.40 0.88 0.81 0.81 0.88 0.84
    Zr 116 119 112 108 114 112 212 233 233 228 246
    Hf 3.34 3.35 3.22 3.05 3.26 3.17 5.78 6.22 6.13 6.14 6.46
    Be 2.24 2.21 2.56 2.14 2.08 2.14 2.16 1.86 1.92 1.74 2.06
    Ga 15.7 16.4 15.7 15.6 15.4 16.1 16.5 16.1 16.4 17.1 16.6
    U 1.16 1.19 1.48 1.15 1.21 1.47 2.68 2.50 2.47 2.73 2.74
    Th 7.26 6.96 6.35 5.64 6.26 6.17 22.6 20.7 19.6 17.7 19.1
    La 22.4 24.4 21.9 17.4 22.3 19.0 69.6 53.7 54.6 54.5 57.8
    Ce 42.2 41.4 41.8 33.1 42.3 39.2 142 109 104 119 124
    Pr 4.12 4.31 4.03 3.32 4.15 3.89 16.0 12.9 13.1 13.8 14.3
    Nd 13.5 14.8 12.8 10.6 13.2 12.5 55.2 47.2 47.2 51.2 51.2
    Sm 2.54 2.51 2.37 1.89 2.35 2.10 9.96 8.84 8.86 9.56 9.51
    Eu 0.95 0.90 0.80 0.71 0.85 0.74 2.44 2.24 2.25 2.34 2.34
    Gd 2.05 2.00 1.83 1.52 1.84 1.62 8.24 7.07 7.20 7.42 7.49
    Tb 0.28 0.28 0.25 0.21 0.25 0.24 1.14 0.98 0.99 0.98 1.07
    Dy 1.32 1.28 1.20 1.02 1.22 1.12 5.39 4.86 4.84 5.01 5.15
    Ho 0.24 0.24 0.22 0.18 0.23 0.21 1.00 0.87 0.88 0.92 0.91
    Er 0.65 0.62 0.55 0.47 0.62 0.56 2.70 2.44 2.42 2.47 2.46
    Tm 0.10 0.09 0.08 0.07 0.09 0.08 0.40 0.37 0.35 0.36 0.35
    Yb 0.60 0.54 0.52 0.44 0.56 0.51 2.46 2.28 2.22 2.13 2.27
    Lu 0.09 0.08 0.08 0.07 0.09 0.08 0.36 0.35 0.34 0.34 0.34
    Y 6.71 5.95 5.54 4.78 5.74 5.51 24.6 21.9 22.3 21.7 22.6
    ΣREE 91.0 93.5 88.4 71.0 90.1 81.9 317 253 249 270 279
    LREE/HREE 16.1 17.2 17.7 16.8 17.4 17.5 13.6 12.2 12.0 12.8 12.9
    (La/Yb)N 26.8 32.4 30.2 28.4 28.6 26.7 20.3 16.9 17.6 18.4 18.3
    δEu 1.23 1.19 1.13 1.24 1.21 1.18 0.80 0.84 0.83 0.82 0.82
    Sr/Y 77.5 97.8 71.5 95.6 91.6 101 28.1 28.1 27.5 31.1 31.2
    La/Yb 37.3 45.2 42.1 39.6 39.8 37.3 28.3 23.6 24.6 25.6 25.5
    Y/Yb 11.2 11.0 10.7 10.9 10.3 10.8 10.0 9.61 10.1 10.2 9.96
    (Ho/Yb)N 3.48 3.87 3.69 3.56 3.58 3.59 3.54 3.32 3.45 3.76 3.49
    Sm/Yb 4.23 4.65 4.56 4.30 4.20 4.12 4.05 3.88 3.99 4.49 4.19
      注:Mg#=100×Mg2+/(Mg2++Fe3+);主量元素含量单位为%,微量和稀土元素含量为10-6
    下载: 导出CSV
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  • 收稿日期:  2017-06-01
  • 修回日期:  2017-07-06
  • 网络出版日期:  2023-08-15
  • 刊出日期:  2018-03-31

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